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Sticking with the formula of the previous seasons that it followed, AYUDHA EZHUTHU Aayudha .New approaches for the investigation of the redox properties and reaction mechanisms of nonheme iron-only proteins.
The recent experimental and theoretical developments in the field of the nonheme iron-only proteins are described, starting with the comparison of the photoinduced and thermal reactivity in the catalytic cycle of myoglobins (Mbs) and cytochromes c (Ccs). The discussion of the excited state behavior of the Mbs is extended and in relation with the results of recent Mossbauer, electrochemical, and EPR studies. The mechanism of the nitrosyl-mediated hydroxylation of terminal alkanes is discussed and some considerations on the role of the iron-ligand interactions in the reactivity are presented. Attention is then turned to the study of iron(II) enzymes that show functional properties very similar to those of Mbs. The properties of mononuclear redox-inactive [(T(2p))Fe(II)Fe(III)(R.S – N(Im(+)))] models, such as the tris(2,2,6,6-tetramethyl-4-piperidinyl)iron (II), the bis(dithiolene)iron complex (Fe(SR)(2)), and the single-molecule complexes [(NH(3))(2)Fe(SR)(2)] and [(H(2)O)Fe(SR)(2)], are described and compared with those of the [(T(2p))Fe(II)Fe(III)(OMe)(NH(3))] derivative, a model for the [(T(2p))Fe(II)Fe(III)(OMe)(OH)] active center, showing high ferrous mononuclear reactivity. A picture for the interactions between the metal ion and the ligand in the above-mentioned iron(II) enzymes is proposed.Milind Kumar Singh Dhakad
Milind Kumar Singh Dhakad (born 1953) is an Indian ophthalmologist and the director of the Synergy Eye Hospital, located in Vashi, Navi Mumbai and Max Super Speciality Eye Hospital, located in Vadgaon, Pune. Singh was the president of the Maharashtra chapter of the Indian Medical Association in 2006 and was awarded the Pravasi Bhart
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